Investigation of the Dispersed-Phase Distribution of Organochlorine Pesticides, Polychlorinated Biphenyls and Polycyclic Aromatic Hydrocarbons in Natural Water Systems

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dc.citation.epage856
dc.citation.issue4
dc.citation.spage846
dc.contributor.affiliationA. V. Dumansky Institute of Colloid Chemistry and Water Chemistry of National Academy of Sciences of Ukraine
dc.contributor.authorMilyukin, Mikhaylo
dc.contributor.authorGorban, Maksym
dc.coverage.placenameЛьвів
dc.coverage.placenameLviv
dc.date.accessioned2025-03-05T08:54:11Z
dc.date.created2023-02-28
dc.date.issued2023-02-28
dc.description.abstractУ статті проаналізовано закономірності дисперсно-фазового розподілу органічних екотоксикантів, а саме: хлорорганічних пестицидів (ХОП), поліхлорованих біфенілів (ПХБ) і поліциклічних ароматичних вуглеводнів (ПАВ) – у природних водних системах. Встановлено залежність між дисперсно-фазовим розподілом індивідуальних ХОП, ПХБ та ПАВ і логарифмом константи розподілу в системі октанол/вода log Ko/w (коефіцієнтом гідрофобності). Показано, що водорозчинна частка індивідуальних органічних екотоксикантів зменшується зі збільшенняи їхнього коефіцієнту гідрофобності. Із одинадцяти наведених кореляцій вісім є чіткими, значимими та достовірними. Також досліджено вплив характеристик водної системи на дисперсно-фазовий розподіл органічних екотоксикантів. Показано, що загальна водорозчинна частка ХОП, ПХБ та ПАВ зменшується зі збільшенням значення хімічного споживання кисню (ХСК), біологічного споживання кисню (БСК) та суми важких металів (Cr, Ni, Cu, Mn, Zn, Cd, Pb). Із дев’яти відповідних кореляцій чотири є чіткими, значимими та достовірними.
dc.description.abstractThe article analyzes the patterns of the dispersed-phase distribution of organic ecotoxicants, namely organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs), and polycyclic aromatic hydrocarbons (PAHs), in natural water systems. The relationship between the dispersed-phase distribution of individual OCPs, PCBs, and PAHs and the logarithm of the octanol-water partition coefficient log Ko/w (hydrophobicity coefficient) was established. It was shown that the water-soluble part of individual organic ecotoxicants decreases with an increase in their hydrophobicity coefficient. Eight of the given eleven correlations are clear, significant and reliable. The influence of the characteristics of the water system on the dispersed-phase distribution of organic ecotoxicants was also investigated. It was shown that the total water-soluble part of OCPs, PCBs, and PAHs decreases with an increase in the chemical oxygen demand (COD), biological oxygen demand (BOD), and the total concentration of heavy metals (Cr, Ni, Cu, Mn, Zn, Cd, Pb). Four of the nine relevant correlations are clear, significant, and reliable.
dc.format.extent846-856
dc.format.pages11
dc.identifier.citationMilyukin M. Investigation of the Dispersed-Phase Distribution of Organochlorine Pesticides, Polychlorinated Biphenyls and Polycyclic Aromatic Hydrocarbons in Natural Water Systems / Mikhaylo Milyukin, Maksym Gorban // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2023. — Vol 17. — No 4. — P. 846–856.
dc.identifier.citationenMilyukin M. Investigation of the Dispersed-Phase Distribution of Organochlorine Pesticides, Polychlorinated Biphenyls and Polycyclic Aromatic Hydrocarbons in Natural Water Systems / Mikhaylo Milyukin, Maksym Gorban // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2023. — Vol 17. — No 4. — P. 846–856.
dc.identifier.doidoi.org/10.23939/chcht17.04.846
dc.identifier.urihttps://ena.lpnu.ua/handle/ntb/63695
dc.language.isoen
dc.publisherВидавництво Львівської політехніки
dc.publisherLviv Politechnic Publishing House
dc.relation.ispartofChemistry & Chemical Technology, 4 (17), 2023
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dc.relation.referencesen[1] Milyukin, M.V.; Goncharuk, V.V. Chemical Monitoring of Organic Ecotoxicants in Water Systems; Naukova dumka: Kyiv, 2016.
dc.relation.referencesen[2] Fiedler, H.; Kallenborn, R.; de Boer, J.; Sydnes, L.K. The Stockholm Convention: A Tool for the Global Regulation of Persistent Organic Pollutants. Chemistry International 2019, 41, 4–11. https://doi.org/10.1515/ci-2019-0202
dc.relation.referencesen[3] Milyukin, M.V.; Goncharuk, V.V. Chemical Monitoring of Organic Ecotoxicants in Aqueous Systems. J. Water Chem. Technol. 2019, 41, 307–312. https://doi.org/10.3103/S1063455X19050060
dc.relation.referencesen[4] Ho, K.T.; Konovets, I.M.; Terletskaya, A.V.; Milyukin, M.V.; Lyashenko, A.V.; Shitikova, L.I.; Shevchuk, L.I.; Afanasiev, S.O.; Krot, Yu.G.; Zorina-Sakharova et al. Contaminants, Mutagenicity and Toxicity in the Surface Waters of Kyiv, Ukraine. Mar. Pollut. Bull. 2020, 155, 111153. https://doi.org/10.1016/j.marpolbul.2020.111153
dc.relation.referencesen[5] Milyukin, M.V.; Gorban, M.V.; Skrynnyk, M.M. Monitoring and Distribution of Organochlorine Pesticides, Polychlorinated Biphenyls and Polycyclic Aromatic Hydrocarbons in Surface River Water and Suspended Particulate Matter. Methods Objects Chem. Anal. 2019, 14, 117–129. https://doi.org/10.17721/moca.2019.117-129
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dc.rights.holder© Національний університет “Львівська політехніка”, 2023
dc.rights.holder© Milyukin M., Gorban M., 2023
dc.subjectХОП
dc.subjectПХБ
dc.subjectПАВ
dc.subjectдисперсно-фазовий розподіл
dc.subjectкоефіцієнт гідрофобності
dc.subjectХСК
dc.subjectБСК
dc.subjectOCPs
dc.subjectPCBs
dc.subjectPAHs
dc.subjectdispersed-phase distribution
dc.subjectcoefficient of hydrophobicity
dc.subjectCOD
dc.subjectBOD
dc.titleInvestigation of the Dispersed-Phase Distribution of Organochlorine Pesticides, Polychlorinated Biphenyls and Polycyclic Aromatic Hydrocarbons in Natural Water Systems
dc.title.alternativeДослідження дисперсно-фазового розподілу хлорорганічних пестицидів, поліхлорованих біфенілів і поліциклічних ароматичних вуглеводнів у природних водних системах
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Chemistry & Chemical Technology. – 2023. – Vol. 17, No. 4