Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues.4. Determining the Optimal Conditions for Tar Modification with Formaldehyde and Properties of the Modified Products

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dc.citation.epage149
dc.citation.issue1
dc.citation.spage142
dc.contributor.affiliationLviv Polytechnic National University
dc.contributor.authorGunka, Volodymyr
dc.contributor.authorBilushchak, Halyna
dc.contributor.authorPrysiazhnyi, Yuriy
dc.contributor.authorDemchuk, Yuriy
dc.contributor.authorHrynchuk, Yurii
dc.contributor.authorSidun, Iurii
dc.contributor.authorShyshchak, Olena
dc.contributor.authorBratychak, Michael
dc.coverage.placenameЛьвів
dc.coverage.placenameLviv
dc.date.accessioned2024-01-22T10:41:30Z
dc.date.available2024-01-22T10:41:30Z
dc.date.created2022-03-16
dc.date.issued2022-03-16
dc.description.abstractДосліджено вплив чинників на перебіг процесу хімічного модифікування гудрону формальдегідом з використанням як каталізатора сульфатної кислоти. Використовуючи експериментальні дані, розроблено адекватну експериментально-статистичну математичну (ЕСМ) модель та на її основі встановлено оптимальні значення чинників процесу хімічного модифікування гудрону формальдегідом з використанням як каталізатора сульфатної кислоти, які забезпечують оптимальні значення пенетрації та температури розм’якшеності модифікованих залишків. Порівняно прогнозовані на основі ЕСМ та практичні дані процесу модифікування залишків.
dc.description.abstractThe effect of factors on the process of chemical modification of tar with formaldehyde using a sulfuric acid as the catalyst has been studied. By using experimental results, the adequate statistical-mathematical (ESM) model has been developed. Based on this model, the optimal values on the process of chemical modification of tar with formaldehyde using a sulfuric acid as the catalyst have been identified, bringing about optimal penetration value and softening point of the modified tars. Data predicted on the basis of the ESM model were compared with empirical evidence about modified tars preparation.
dc.format.extent142-149
dc.format.pages8
dc.identifier.citationProduction of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues.4. Determining the Optimal Conditions for Tar Modification with Formaldehyde and Properties of the Modified Products / Volodymyr Gunka, Halyna Bilushchak, Yuriy Prysiazhnyi, Yuriy Demchuk, Yurii Hrynchuk, Iurii Sidun, Olena Shyshchak, Michael Bratychak // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2022. — Vol 16. — No 1. — P. 142–149.
dc.identifier.citationenProduction of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues.4. Determining the Optimal Conditions for Tar Modification with Formaldehyde and Properties of the Modified Products / Volodymyr Gunka, Halyna Bilushchak, Yuriy Prysiazhnyi, Yuriy Demchuk, Yurii Hrynchuk, Iurii Sidun, Olena Shyshchak, Michael Bratychak // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2022. — Vol 16. — No 1. — P. 142–149.
dc.identifier.doidoi.org/10.23939/chcht16.01.142
dc.identifier.urihttps://ena.lpnu.ua/handle/ntb/60951
dc.language.isoen
dc.publisherВидавництво Львівської політехніки
dc.publisherLviv Politechnic Publishing House
dc.relation.ispartofChemistry & Chemical Technology, 1 (16), 2022
dc.relation.references[1] Muneraa, J.C.; Ossa, E.A. Polymer Modified Bitumen: Optimization and Selection. Mater. Design2016, 62, 91-97.https://doi.org/10.1016/j.matdes.2014.05.009
dc.relation.references[2] Pyshyev, S.;Gunka, V.;Grytsenko, Yu.; Bratychak, M. Polymer Modified Bitumen: Review. Chem. Chem. Technol. 2016, 10 (4s), 631-636. https://doi.org/10.23939/chcht10.04si.631
dc.relation.references[3] Gorkem, C., Sengoz, B. Predicting Stripping and Moisture Induced Damage of Asphalt Concrete Prepared with Polymer Modified Bitumen and Hydrated Lime. Constr. Build. Mater.2009, 23 (6), 2227-2236.https://doi.org/10.1016/j.conbuildmat.2008.12.001
dc.relation.references[4] Brozyna, D., Kowalski, K.J. Assestment of Polyethylene-Modified Bitumen Adhesion Using Computer Image Analysis. Arch. Civ. Eng.2016, LXII (4), 3-18.https://doi.org/10.1515/ace-2015-0106
dc.relation.references[5] Zielinski, K.; Babiak, M.; Ratajczak, M.; Kosno, J. Impact of Chemical and Physical Modification on Thermoplastic Characteristics of Bitumen. Procedia Eng. 2017, 172, 1297-1304.https://doi.org/10.1016/j.proeng.2017.02.159
dc.relation.references[6] Nagurskyy, A.; Khlibyshyn, Y.; Grynyshyn, O.; Kochubei, V. Rubber Crumb Modified Bitumen Produced from Crude Oil Residuals of Ukrainian Deposits.Chem. Chem. Technol.2020, 14 (4) 420-425. https://doi.org/10.23939/chcht14.03.420
dc.relation.references[7] Ibrahim, M. R.;Katman, H. Y.; Karim, M. R.;Koting, S.;Mashaan, N. S. A Review on the Effect of Crumb Rubber Addition to the Rheology of Crumb Rubber Modified Bitumen. Adv.Mater. Sci. Eng. 2013, 2013,1-8. https://doi.org/10.1155/2013/415246
dc.relation.references[8] Bratychak, M.;Chervinskyy, T.;Astakhova, O.; Shyshchak, O.Bitumen Production via Tar Oxidation in the Presence of Petroleum Resin with Fluorine-Containing Groups. Chem. Chem. Technol. 2010, 4, 325-328. https://doi.org/10.23939/chcht04.04.325
dc.relation.references[9] Grynyshyn, O.;Bratychak, M.;Krynytskiy, V.; Donchak, V. Petroleum Resins for Bitumens Modification. Chem. Chem. Technol. 2008, 2, 47-53.https://doi.org/10.23939/chcht02.01.047
dc.relation.references[10] Strap, G.;Astakhova, O.;Lazorko, O.; Shyshchak, O.; Bratychak, M.Modified Phenol-Formaldehyde Resins and Their Application in Bitumen-Polymeric Mixtures. Chem. Chem. Technol. 2013, 7, 279-287. https://doi.org/10.23939/chcht07.03.279
dc.relation.references[11] Bratychak, M.;Iatsyshyn, O.;Shyshchak, O.; Astakhova, O.; Janik, H.Carboxy Derivative of DioxydiphenylpropaneDiglycidyl Ether Monomethacrylate as an Additive for Composites.Chem. Chem. Technol, 2017, 11, 49-54. https://doi.org/10.23939/chcht11.01.049
dc.relation.references[12] Sidun, I.;Solodkyy, S.; Shved, M.; Astakhova, O.; Shyshchak, O.; Bratychak, M.Obtaining of Coumarone-Indene Resins based on Light Fraction of Coal Tar. 5. Emulsions on the Basis of Bitumen Modified by Coumarone-Indene Resins with Epoxy Groups. Chem. Chem. Technol.2019, 13, 489-494. https://doi.org/10.23939/chcht13.04.489
dc.relation.references[13] Demchuk, Y.;Gunka, V.;Pyshyev, S.; Sidun, I.; Hrynchuk, Y.; Kucinska-Lipka, J.; Bratychak, M.Slurry Surfacing Mixes on the Basis of Bitumen Modified with Phenol-Cresol-Formaldehyde Resin. Chem. Chem. Technol. 2020, 14, 251-256. https://doi.org/10.23939/chcht14.02.251
dc.relation.references[14] Demchuk, Y.;Gunka, V.;Sidun, I.;Solodkyy, S. Comparison of Bitumen Modified by Phenol Formaldehyde Resins Synthesized from Different Raw Materials.Proc. of EcoComfort.2020, 100, 95-102https://doi.org/10.1007/978-3-030-57340-9_1
dc.relation.references[15] Gunka, V.;Demchuk, Y.;Sidun, I.;Miroshnichenko, D.;Nyakuma, B.B.; Pyshyev, S. Application of phenol-cresol-formaldehyde resin as an adhesion promoter for bitumen and asphalt concrete. Road Mater. Pavement Des.2020, 22(12),2906-2918.https://doi.org/10.1080/14680629.2020.1808518
dc.relation.references[16] Bratychak, M.; Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 1. Effect of Solvent Nature on the Properties of Petroleum Residues Modified with Folmaldehyde.Chem. Chem. Technol. 2021, 15 (2), 274-283. https://doi.org/10.23939/chcht15.02.274
dc.relation.references[17] Gunka, V.; Demchuk, Y.; Sidun, I.; Kochubei, V.; Shved. M.;Romanchuk, V.; Korchak, B. Chemical modification of road oil bitumens by formaldehyde.Pet. Coal.2020, 62(1), 420-429.
dc.relation.references[18] Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O.; Bratychak, M. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 2. Bitumen Modified with Maleic Anhydride. Chem. Chem. Technol. 2021, 15 (3), 443-449. https://doi.org/10.23939/chcht15.03.443
dc.relation.references[19] Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O.; Poliak, O.; Bratychak, M. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 2. Tar Modified with Formaldehyde. Chem. Chem. Technol. 2021, 15 (4), 608-620.https://doi.org/10.23939/chcht15.04.608
dc.relation.references[20] Singh, B.; Lokesh, K.; Gupta, M.; Chauhan, G.S. Polymer-Modified Bitumen of Recycled LDPE and Maleated Bitumen. J. Appl. Polym. Sci.2013, 127, 67-78. https://doi.org/10.1002/app.36810
dc.relation.references[21] Tsegelyk, G.G. OsnovyEkonometrii; Vydavnutsvo LNU im. Franka: Lviv, 2011.
dc.relation.references[22] Bolshev, L.N.; Smirnov, N.B. TablitsyMatematicheskoiStatistiki; Nauka: Moskva, 1983.
dc.relation.referencesen[1] Muneraa, J.C.; Ossa, E.A. Polymer Modified Bitumen: Optimization and Selection. Mater. Design2016, 62, 91-97.https://doi.org/10.1016/j.matdes.2014.05.009
dc.relation.referencesen[2] Pyshyev, S.;Gunka, V.;Grytsenko, Yu.; Bratychak, M. Polymer Modified Bitumen: Review. Chem. Chem. Technol. 2016, 10 (4s), 631-636. https://doi.org/10.23939/chcht10.04si.631
dc.relation.referencesen[3] Gorkem, C., Sengoz, B. Predicting Stripping and Moisture Induced Damage of Asphalt Concrete Prepared with Polymer Modified Bitumen and Hydrated Lime. Constr. Build. Mater.2009, 23 (6), 2227-2236.https://doi.org/10.1016/j.conbuildmat.2008.12.001
dc.relation.referencesen[4] Brozyna, D., Kowalski, K.J. Assestment of Polyethylene-Modified Bitumen Adhesion Using Computer Image Analysis. Arch. Civ. Eng.2016, LXII (4), 3-18.https://doi.org/10.1515/ace-2015-0106
dc.relation.referencesen[5] Zielinski, K.; Babiak, M.; Ratajczak, M.; Kosno, J. Impact of Chemical and Physical Modification on Thermoplastic Characteristics of Bitumen. Procedia Eng. 2017, 172, 1297-1304.https://doi.org/10.1016/j.proeng.2017.02.159
dc.relation.referencesen[6] Nagurskyy, A.; Khlibyshyn, Y.; Grynyshyn, O.; Kochubei, V. Rubber Crumb Modified Bitumen Produced from Crude Oil Residuals of Ukrainian Deposits.Chem. Chem. Technol.2020, 14 (4) 420-425. https://doi.org/10.23939/chcht14.03.420
dc.relation.referencesen[7] Ibrahim, M. R.;Katman, H. Y.; Karim, M. R.;Koting, S.;Mashaan, N. S. A Review on the Effect of Crumb Rubber Addition to the Rheology of Crumb Rubber Modified Bitumen. Adv.Mater. Sci. Eng. 2013, 2013,1-8. https://doi.org/10.1155/2013/415246
dc.relation.referencesen[8] Bratychak, M.;Chervinskyy, T.;Astakhova, O.; Shyshchak, O.Bitumen Production via Tar Oxidation in the Presence of Petroleum Resin with Fluorine-Containing Groups. Chem. Chem. Technol. 2010, 4, 325-328. https://doi.org/10.23939/chcht04.04.325
dc.relation.referencesen[9] Grynyshyn, O.;Bratychak, M.;Krynytskiy, V.; Donchak, V. Petroleum Resins for Bitumens Modification. Chem. Chem. Technol. 2008, 2, 47-53.https://doi.org/10.23939/chcht02.01.047
dc.relation.referencesen[10] Strap, G.;Astakhova, O.;Lazorko, O.; Shyshchak, O.; Bratychak, M.Modified Phenol-Formaldehyde Resins and Their Application in Bitumen-Polymeric Mixtures. Chem. Chem. Technol. 2013, 7, 279-287. https://doi.org/10.23939/chcht07.03.279
dc.relation.referencesen[11] Bratychak, M.;Iatsyshyn, O.;Shyshchak, O.; Astakhova, O.; Janik, H.Carboxy Derivative of DioxydiphenylpropaneDiglycidyl Ether Monomethacrylate as an Additive for Composites.Chem. Chem. Technol, 2017, 11, 49-54. https://doi.org/10.23939/chcht11.01.049
dc.relation.referencesen[12] Sidun, I.;Solodkyy, S.; Shved, M.; Astakhova, O.; Shyshchak, O.; Bratychak, M.Obtaining of Coumarone-Indene Resins based on Light Fraction of Coal Tar. 5. Emulsions on the Basis of Bitumen Modified by Coumarone-Indene Resins with Epoxy Groups. Chem. Chem. Technol.2019, 13, 489-494. https://doi.org/10.23939/chcht13.04.489
dc.relation.referencesen[13] Demchuk, Y.;Gunka, V.;Pyshyev, S.; Sidun, I.; Hrynchuk, Y.; Kucinska-Lipka, J.; Bratychak, M.Slurry Surfacing Mixes on the Basis of Bitumen Modified with Phenol-Cresol-Formaldehyde Resin. Chem. Chem. Technol. 2020, 14, 251-256. https://doi.org/10.23939/chcht14.02.251
dc.relation.referencesen[14] Demchuk, Y.;Gunka, V.;Sidun, I.;Solodkyy, S. Comparison of Bitumen Modified by Phenol Formaldehyde Resins Synthesized from Different Raw Materials.Proc. of EcoComfort.2020, 100, 95-102https://doi.org/10.1007/978-3-030-57340-9_1
dc.relation.referencesen[15] Gunka, V.;Demchuk, Y.;Sidun, I.;Miroshnichenko, D.;Nyakuma, B.B.; Pyshyev, S. Application of phenol-cresol-formaldehyde resin as an adhesion promoter for bitumen and asphalt concrete. Road Mater. Pavement Des.2020, 22(12),2906-2918.https://doi.org/10.1080/14680629.2020.1808518
dc.relation.referencesen[16] Bratychak, M.; Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 1. Effect of Solvent Nature on the Properties of Petroleum Residues Modified with Folmaldehyde.Chem. Chem. Technol. 2021, 15 (2), 274-283. https://doi.org/10.23939/chcht15.02.274
dc.relation.referencesen[17] Gunka, V.; Demchuk, Y.; Sidun, I.; Kochubei, V.; Shved. M.;Romanchuk, V.; Korchak, B. Chemical modification of road oil bitumens by formaldehyde.Pet. Coal.2020, 62(1), 420-429.
dc.relation.referencesen[18] Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O.; Bratychak, M. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 2. Bitumen Modified with Maleic Anhydride. Chem. Chem. Technol. 2021, 15 (3), 443-449. https://doi.org/10.23939/chcht15.03.443
dc.relation.referencesen[19] Gunka, V.; Prysiazhnyi, Yu.; Hrynchuk, Yu.; Sidun, I.; Demchuk, Yu.; Shyshchak, O.; Poliak, O.; Bratychak, M. Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 2. Tar Modified with Formaldehyde. Chem. Chem. Technol. 2021, 15 (4), 608-620.https://doi.org/10.23939/chcht15.04.608
dc.relation.referencesen[20] Singh, B.; Lokesh, K.; Gupta, M.; Chauhan, G.S. Polymer-Modified Bitumen of Recycled LDPE and Maleated Bitumen. J. Appl. Polym. Sci.2013, 127, 67-78. https://doi.org/10.1002/app.36810
dc.relation.referencesen[21] Tsegelyk, G.G. OsnovyEkonometrii; Vydavnutsvo LNU im. Franka: Lviv, 2011.
dc.relation.referencesen[22] Bolshev, L.N.; Smirnov, N.B. TablitsyMatematicheskoiStatistiki; Nauka: Moskva, 1983.
dc.relation.urihttps://doi.org/10.1016/j.matdes.2014.05.009
dc.relation.urihttps://doi.org/10.23939/chcht10.04si.631
dc.relation.urihttps://doi.org/10.1016/j.conbuildmat.2008.12.001
dc.relation.urihttps://doi.org/10.1515/ace-2015-0106
dc.relation.urihttps://doi.org/10.1016/j.proeng.2017.02.159
dc.relation.urihttps://doi.org/10.23939/chcht14.03.420
dc.relation.urihttps://doi.org/10.1155/2013/415246
dc.relation.urihttps://doi.org/10.23939/chcht04.04.325
dc.relation.urihttps://doi.org/10.23939/chcht02.01.047
dc.relation.urihttps://doi.org/10.23939/chcht07.03.279
dc.relation.urihttps://doi.org/10.23939/chcht11.01.049
dc.relation.urihttps://doi.org/10.23939/chcht13.04.489
dc.relation.urihttps://doi.org/10.23939/chcht14.02.251
dc.relation.urihttps://doi.org/10.1007/978-3-030-57340-9_1
dc.relation.urihttps://doi.org/10.1080/14680629.2020.1808518
dc.relation.urihttps://doi.org/10.23939/chcht15.02.274
dc.relation.urihttps://doi.org/10.23939/chcht15.03.443
dc.relation.urihttps://doi.org/10.23939/chcht15.04.608
dc.relation.urihttps://doi.org/10.1002/app.36810
dc.rights.holder© Національний університет “Львівська політехніка”, 2022
dc.rights.holder© Gunka V., Bilushchak H., Prysiazhnyi Y., Demchuk Y., Hrynchuk Y., Sidun I., Shyshchak O., Bratychak M., 2022
dc.subjectгудрон
dc.subjectформальдегід
dc.subjectоптимальні умови
dc.subjectекспериментально-статистична математична модель
dc.subjecttar
dc.subjectformaldehyde
dc.subjectoptimal conditions
dc.subjectexperimental statistical-mathematical (ESM) model
dc.titleProduction of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues.4. Determining the Optimal Conditions for Tar Modification with Formaldehyde and Properties of the Modified Products
dc.title.alternativeОдержання бітуму, модифікованого низькомолекулярними органічними сполуками із нафтових залишків. 4. Встановлення оптимальних умов процесу модифікування гудрону формальдегідом та властивості модифікованих продуктів
dc.typeArticle

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Chemistry & Chemical Technology. – 2022. – Vol. 16, No. 1