Samarium-doped ceria/yttria-stabilized zirconia composite prepared by solid state reaction

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dc.citation.epage440
dc.citation.issue4
dc.citation.journalTitleChemistry & Chemical Technology
dc.citation.spage434
dc.citation.volume12
dc.contributor.affiliationResearch Group of Solid State Chemistry & Catalysis, Chemistry Department, Sebelas Maret University, Indonesia
dc.contributor.affiliationCeramics Lab., National Atomic Energy Agency, Badan Tenaga Atom
dc.contributor.affiliationNasional (BATAN), Jl. Taman Sari Bandung, Indonesia
dc.contributor.authorRahmawati, Fitria
dc.contributor.authorRespati, Anang Pandan
dc.contributor.authorMudjijono
dc.contributor.authorSyarif, Dani G.
dc.coverage.placenameLviv
dc.date.accessioned2019-06-21T07:58:01Z
dc.date.available2019-06-21T07:58:01Z
dc.date.created2018-01-20
dc.date.issued2018-01-20
dc.description.abstractОдержано композити с різним співвідно- шенням промотованого самарієм оксиду церію (SDC) з діоксидом цирконію, стабілізованого оксидом ітрію (YSZ), SDC:YSZ = 0:1; 1:9; 1:1; 9:1 та 1:0. Досліджено структуру кристалів та йонну провідність одержаних композитів. За допомогою рентгенодифракційного аналізу з використанням методу Ле Бейля досліджено кристалічну структуру, просторові групи, параметри та об‘єм комірок. Йонну провідність визначено методом імпедансу. Показано, що композити SDC-YSZ кристалізувались у двох фазаз кубічного SDC і кубічного YSZ за відсутності вторинних фаз. Це вказує на те, що змішування та нагрівання за 1523 К не змінюють кристалічну структуру, навіть при зміні параметрів комірки. Композит SDC-YSZ 91 показує найвищу йонну провідність за 873 К. Показана роль YSZ щодо гальмування автовідновлення йонів церію.
dc.description.abstract1A research on the preparation of composite samarium-doped ceria (SDC) with yttrium-stabilized zirconia (YSZ) has been conducted at the SDC:YSZ ratio of 0:1; 1:9; 1:1; 9:1 and 1:0. This research aims to investigate the crystal structure and the ionic conductivity of the prepared materials. XRD analysis equipped with Le Bail refinement was used to analyze the crystal structure, space group, cell parameters, and cell volume. Meanwhile, the ionic conductivity was determined by impedance measurement. The result shows that the composites of SDC-YSZ were crystallized in two phases of cubic SDC and cubic YSZ without the presence of secondary phases. It indicates that the mixing and the heating at 1523 K did not change the crystal structure, even though it changed the cell parameters. Composite SDC-YSZ 91 shows a highest ionic conductivity at 873K without the presence of electrode-bulk interface conductivity. It is a good indication of YSZ role regarding the inhibition of cerium ions auto-reduction.
dc.format.extent434-440
dc.format.pages7
dc.identifier.citationSamarium-doped ceria/yttria-stabilized zirconia composite prepared by solid state reaction / Fitria Rahmawati, Anang Pandan Respati, Mudjijono, Dani G. Syarif // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2018. — Vol 12. — No 4. — P. 434–440.
dc.identifier.citationenSamarium-doped ceria/yttria-stabilized zirconia composite prepared by solid state reaction / Fitria Rahmawati, Anang Pandan Respati, Mudjijono, Dani G. Syarif // Chemistry & Chemical Technology. — Lviv : Lviv Politechnic Publishing House, 2018. — Vol 12. — No 4. — P. 434–440.
dc.identifier.urihttps://ena.lpnu.ua/handle/ntb/45207
dc.language.isoen
dc.publisherLviv Politechnic Publishing House
dc.relation.ispartofChemistry & Chemical Technology, 4 (12), 2018
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dc.relation.urihttps://doi.org/10.1038/35104620
dc.relation.urihttps://doi.org/
dc.relation.urihttps://doi.org/10.1016/j.ssi.2004.07.042
dc.relation.urihttps://doi.org/10.1039/b612060c
dc.relation.urihttp://dx.doi.org/10.1063/1.4943447
dc.relation.urihttps://doi.org/10.1016/S0167-2738(99)00319-7
dc.relation.urihttps://doi.org/10.1016/j.pmatsci.2005.07.001
dc.relation.urihttps://doi.org/10.1016/0167-2738(95)00229-4
dc.relation.urihttps://doi.org/10.1016/j.ssi.2004.03.034
dc.relation.urihttps://doi.org/10.1016/j.elecom.2007.07.036
dc.relation.urihttps://doi.org/10.1016/j.ijhydene.2010.01.063
dc.relation.urihttps://doi.org/10.1016/j.ijhydene.2013.10.096
dc.relation.urihttps://doi.org/10.1016/j.materresbull.2006.04.001
dc.relation.urihttps://doi.org/10.1016/j.compscitech.2009.10.006
dc.relation.urihttps://doi.org/10.1016/j.jpowsour.2013.01.138
dc.relation.urihttps://doi.org/10.1149/1.1838378
dc.relation.urihttps://doi.org/10.1007/s10853-014-8265-5
dc.relation.urihttps://doi.org/10.1016/j.ceramint.2014.11.131
dc.relation.urihttps://doi.org/10.1016/j.ssi.2004.09.040
dc.relation.urihttps://doi.org/10.1557/jmr.2006.0041
dc.relation.urihttps://doi.org/10.1149/1.3432253
dc.relation.urihttps://doi.org/10.1016/j.solidstatesciences.2007.03.023
dc.relation.urihttps://doi.org/10.1149/1.1846711
dc.relation.urihttps://doi.org/10.1016/S0254-0584(01)00522-3
dc.relation.urihttps://doi.org/10.1149/1.2129007
dc.rights.holder© Національний університет „Львівська політехніка“, 2018
dc.rights.holder©Rahmawati F., Respati A., Mudjijono, Syarif D., 2018
dc.subjectкомпозит SDC-YSZ
dc.subjectелектроліт
dc.subjectтвердооксидний паливний елемент
dc.subjectйонна провідність
dc.subjectSDC-YSZ composite
dc.subjectelectrolyte
dc.subjectsolid oxide fuel cell
dc.subjectionic conductivity
dc.titleSamarium-doped ceria/yttria-stabilized zirconia composite prepared by solid state reaction
dc.title.alternativeОдержання за реакцією у твердому стані композиту промотованого самарієм оксид церію/діоксид цирконію, стабілізованого оксидом ітрію
dc.typeArticle

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Chemistry & Chemical Technology. – 2018. – Vol. 12, No. 4